Browsing by Author "Giraud, Robert J."
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Item Combustion operating conditions for municipal Waste-to-Energy facilities in the U.S.(Waste Management, 2021-08-01) Giraud, Robert J.; Taylor, Philip H.; Huang, Chin-paoHighlights • Survey of U.S. municipal waste-to-energy (WTE) facilities identified 188 boilers. • These WTE boilers were stratified into nine categories by combustion technology. • WTE boilers typically operate at a gas residence time > 2.4 s above 1160°C. Abstract This paper reports the first known comprehensive survey of combustion operating conditions across the wide range of municipal waste-to-energy facilities in the U.S. The survey was conducted in a step-wise fashion. Once the population of 188 units operating at over 70 facilities was defined, this population was stratified by distinguishing characteristics of combustion technology. Stratum-level estimates for operating conditions were determined from data collected in the survey. These stratum-level values were weighted by corresponding design capacity share and combined to infer national-level operating parameter estimates representative of the overall population. Survey results show that typical municipal waste-to-energy combustion operating conditions in the U.S. are (1) furnace temperature above 1160 °C, (2) gas residence time above 2.4 s, (3) exit gas concentrations of nearly 10% for oxygen (dry basis), and (4) over 16% for moisture. These operating parameter values can serve as benchmarks for laboratory-scale studies representative of municipal waste-to-energy combustion as typically practiced in the U.S. Graphical abstract Available at: https://doi.org/10.1016/j.wasman.2021.07.015Item Design and qualification of a bench-scale model for municipal waste-to-energy combustion(Journal of the Air & Waste Management Association, 2022-04-25) Giraud, Robert J.; Taylor, Philip H.; Diemer, R. Bertrum; Huang, Chin-PaoThis paper reports the design and qualification of the first purpose-built, bench-scale reactor system to model the municipal waste-to-energy combustion of fluorinated polymers. Using the principle of similarity, the gas-phase combustion zone of a typical municipal waste-to-energy plant has been scaled down to the bench with a focus on chemical similarity. Chemical similarity is achieved in large part through the use of methanol as a surrogate for municipal solid waste (MSW). Review of prior research shows that methanol is one of the major volatile products expected during MSW thermal conversion in the fuel bed of waste-to-energy plants. Like full-scale waste-energy plants, the design of the bench-scale model includes a flame zone and a post-flame zone. Maintaining steady methanol vapor flow premixed with air to the model reactor system ensures stable combustion resulting in bench-scale CO emission levels comparable to those of full-scale waste-to-energy plants. Since investigation of fluorinated polymer combustion includes trace analysis of exhaust gas for perfluorooctanoic acid (PFOA), qualification testing focused on PFOA collection efficiency. High PFOA collection efficiency (>90%) demonstrated the capability of the reactor system in transporting and absorbing PFOA that may be generated during high-temperature combustion testing of fluorinated polymers. Overall, the bench-scale system is qualified for its intended use to investigate potential generation of PFOA from combustion of fluorinated polymers under conditions representative of waste-to-energy combustion. Implications: Decision makers depend on environmental researchers to provide reliable predictions of pollutant emissions from waste combustion of polymers at end of product life. Reliable predictions are especially important with regard to questions about potential PFOA emissions from municipal waste combustion of fluorinated polymers. Results from qualification testing confirm that the novel bench-scale model reactor system is capable of representing gas-phase municipal waste combustion behavior upstream of air pollution control and generating representative exhaust gas samples for off-line trace-level analysis of PFOA.