Quantification of Lignin Degradation Products in Dissolved Organic Matter Among Three Tree Species

Date
2024-05
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University of Delaware
Abstract
Stemflow is a major source of dissolved organic matter (DOM) into the subsoil around a tree via preferential flow paths. Contained in the DOM matrix is soluble lignin which is an aromatic polymer that is an important structural component of terrestrial plants, resistant to microbial and environmental degradation and can serve as a powerful biomarker. Numerous studies have been conducted quantifying lignin content in DOM derived from surface waters globally, but none exist on stemflow. In this study, samples from Liriodendron tuliprifera L. (yellow poplar), Fagus grandifolia Ehrh (American beech), and Betula lenta L. (sweet birch) were collected and lignin isolated by solid phase extraction for my experiments. Ultraviolet-visible light and fluorescence spectrometry was conducted alongside high performance liquid chromatography mass spectrometry to quantify lignin in stemflow DOM. In this study, it was observed that normalized lignin concentrations were an order of magnitude greater than those measured in freshwater systems demonstrating the importance of stemflow DOM as a major source of soluble lignin into the subsoil. This study also overlapped a large Canadian wildfire in 2023 and found some evidence that stemflow DOM composition was affected by these wildfires.
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